Presentation 1993/5/24
Nonlinear optical spectroscopy of one dimensional excitons in polysilanes
Hideo Kishida, Tatsuo Hasegawa, Yoshihiro Iwasa, Takao Koda, Yoshinori Tokura, Hiroaki Tachibana,
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Abstract(in English) Polysilanes,whose backbones consist of silicn atoms,is known to have one-dimensional delocaized electronic states.We have evaluated nonlinear optical susceptibilities of thin films of polysilanes by measurements of third-harmonic generation and electric-field induced second-harmonic generation.Comparing the results with the one-photon and two-photon absorption spectra,we found that one-dimensional excitons do exist with a series of quantum numbers and play essential roles in the nonlinear process in polysilanes.Novel features of one-dimensional excitons are discussed by analysis of the spectroscopic results in terms of the theoretical model.
Keyword(in Japanese) (See Japanese page)
Keyword(in English) polysilane / third-harmonic generation / electric-field induced second harmonic generation / one-dimensional exciton / third- order nonlinear susceptibility
Paper # OME93-2
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Committee OME
Conference Date 1993/5/24(1days)
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Registration To Organic Material Electronics (OME)
Language JPN
Title (in Japanese) (See Japanese page)
Sub Title (in Japanese) (See Japanese page)
Title (in English) Nonlinear optical spectroscopy of one dimensional excitons in polysilanes
Sub Title (in English)
Keyword(1) polysilane
Keyword(2) third-harmonic generation
Keyword(3) electric-field induced second harmonic generation
Keyword(4) one-dimensional exciton
Keyword(5) third- order nonlinear susceptibility
1st Author's Name Hideo Kishida
1st Author's Affiliation Department of Applied Physics,Faculty of Engineering,University of Tokyo()
2nd Author's Name Tatsuo Hasegawa
2nd Author's Affiliation Department of Applied Physics,Faculty of Engineering,University of Tokyo
3rd Author's Name Yoshihiro Iwasa
3rd Author's Affiliation Department of Applied Physics,Faculty of Engineering,University of Tokyo
4th Author's Name Takao Koda
4th Author's Affiliation Department of Applied Physics,Faculty of Engineering,University of Tokyo
5th Author's Name Yoshinori Tokura
5th Author's Affiliation Department of Physics,Faculty of Science,University of Tokyo
6th Author's Name Hiroaki Tachibana
6th Author's Affiliation National Institute of Materials and Chemical Research
Date 1993/5/24
Paper # OME93-2
Volume (vol) vol.93
Number (no) 61
Page pp.pp.-
#Pages 6
Date of Issue